| DOI | Trouver le DOI : https://doi.org/10.1126/science.1169183 |
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| Auteur | Rechercher : Bisgaard, Christer Z.1; Rechercher : Clarkin, Owen J.1; Rechercher : Wu, Guorong2; Rechercher : Lee, Anthony M. D.1; Rechercher : Geßner, Oliver; Rechercher : Hayden, Carl C.; Rechercher : Stolow, Albert1 |
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| Affiliation | - Conseil national de recherches du Canada. Institut Steacie des sciences moléculaires du CNRC
- Conseil national de recherches du Canada. Institut de biotechnologie des plantes du CNRC
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| Format | Texte, Article |
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| Sujet | molecules; dynamic imaging; molecular structures; ultrafast; photochemical |
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| Résumé | Random orientation of molecules within a sample leads to blurred observations of chemical reactions studied from the laboratory perspective. Methods developed for the dynamic imaging of molecular structures and processes struggle with this, as measurements are optimally made in the molecular frame. We used laser alignment to transiently fix carbon disulfide molecules in space long enough to elucidate, in the molecular reference frame, details of ultrafast electronic-vibrational dynamics during a photochemical reaction. These three-dimensional photoelectron imaging results, combined with ongoing efforts in molecular alignment and orientation, presage a wide range of insights obtainable from time-resolved studies in the molecular frame. |
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| Date de publication | 2009-03-13 |
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| Dans | |
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| Langue | anglais |
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| Publications évaluées par des pairs | Oui |
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| Numéro NPARC | 16488520 |
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| Exporter la notice | Exporter en format RIS |
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| Signaler une correction | Signaler une correction (s'ouvre dans un nouvel onglet) |
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| Identificateur de l’enregistrement | 11f46791-077f-43ad-abcd-dd7a6490ef33 |
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| Enregistrement créé | 2011-02-15 |
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| Enregistrement modifié | 2020-04-16 |
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