DOI | Resolve DOI: https://doi.org/10.1038/35107000 |
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Author | Search for: Hentschel, M.; Search for: Kienberger, R.; Search for: Spielmann, Ch; Search for: Reider, G.; Search for: Milosevic, N.; Search for: Brabec, T.; Search for: Corkum, P.1; Search for: Heinzmann, U.; Search for: Drescher, M.; Search for: Krausz, F. |
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Affiliation | - National Research Council of Canada. NRC Steacie Institute for Molecular Sciences
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Format | Text, Article |
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Abstract | The generation of ultrashort pulses is a key to exploring the dynamic behaviour of matter on ever-shorter timescales. Recent developments have pushed the duration of laser pulses close to its natural limit�the wave cycle, which lasts somewhat longer than one femtosecond (1 fs = 10-15 s) in the visible spectral range. Time-resolved measurements with these pulses are able to trace dynamics of molecular structure, but fail to capture electronic processes occurring on an attosecond (1 as = 10-18 s) timescale. Here we trace electronic dynamics with a time resolution of less than or equal to 150 as by using a subfemtosecond soft-X-ray pulse and a few-cycle visible light pulse. Our measurement indicates an attosecond response of the atomic system, a soft-X-ray pulse duration of 650 plusminus 150 as and an attosecond synchronism of the soft-X-ray pulse with the light field. The demonstrated experimental tools and techniques open the door to attosecond spectroscopy of bound electrons. |
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Publication date | 2001-11-29 |
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In | |
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Language | English |
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Peer reviewed | Yes |
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NPARC number | 12328272 |
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Export citation | Export as RIS |
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Report a correction | Report a correction (opens in a new tab) |
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Record identifier | e6f7252e-e1ca-48b8-8388-0049e9a1fba5 |
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Record created | 2009-09-10 |
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Record modified | 2020-03-27 |
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